Study of the Pickering emulsion stabilizing ability of deep eutectic solvent–ultra high pressure homogenization processed nanocellulose [* Cross-Reference *]

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You, Lingxin; Fischer, Peter; Soukoulis, Christos, 2026, "Study of the Pickering emulsion stabilizing ability of deep eutectic solvent–ultra high pressure homogenization processed nanocellulose [* Cross-Reference *]", https://lore.list.lu/citation?persistentId=perma:LIST.CTFR91, LIST Open Repository, V1
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Description
Nanocelluloses are versatile, bio-based materials capable of forming stable colloidal systems via Pickering stabilization. The combination of deep eutectic solvent (DES) pretreatment with ultra-high-pressure homogenization (UHPH) represents a promising green strategy to produce functional nanocellulose particles with tunable properties. In the present work, choline chloride-based DESs with glycerol (Ch_G), urea (Ch_U), or malic acid (Ch_MA) were used to pretreat microcrystalline cellulose prior to UHPH processing, yielding nanocelluloses with distinct morphologies and surface characteristics. Pickering oil-in-water emulsions were prepared, and their microstructure, rheological behavior, and colloidal stability were evaluated under varying temperature, pH, and ionic strength conditions. Ch_G and Ch_U treated nanocellulose exhibited long, flexible fibrils that stabilized the o/w emulsions primarily through network-mediated steric hindrance and lipid droplet immobilization. In contrast, Ch_MA treated nanocellulose featured shorter, highly charged particles that enhanced droplet dispersion via electrostatic repulsion though showing higher sensitivity to pH and ionic strength. Overall, the Pickering o/w emulsions demonstrated high stability over a broad range of temperatures (25–50 °C), pH values (4.5–10), and ionic strengths (≤ 200 mM NaCl), highlighting the effectiveness of DES–UHPH processing for tuning nanocellulose-based Pickering stabilization mechanisms in food-relevant emulsion systems. (2026-05-01)
***This entry has been automatically imported via Infodoc(ASO) CSV by LIST harvest scripts. Please refer to https://doi.org/10.1016/j.foodres.2026.118758 for the original and latest version of the dataset and data downloads*** (2026-06-04)
Subject Earth and Environmental Sciences
Keyword Colloidal stability, Electrostatic and steric interactions, Interfacial stabilization, Nanocellulose, Oil-in-water emulsions, Pickering particles
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