Understanding Plasma–Liquid Interactions and Plasma‐Induced Free‐Radical Polymerisation in Liquid‐Assisted Atmospheric Plasma Polymerisation—Application to Antioxidant Coating [* Cross-Reference *]

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Angelica Maria Lanza; Kamal Baba; François Loyer; Lotfi Boudjema; Riadh Bourzami; Fabio Palumbo; Pietro Favia; Nicolas D. Boscher, 2026, "Understanding Plasma–Liquid Interactions and Plasma‐Induced Free‐Radical Polymerisation in Liquid‐Assisted Atmospheric Plasma Polymerisation—Application to Antioxidant Coating [* Cross-Reference *]", https://lore.list.lu/citation?persistentId=perma:LIST.AKHJTS, LIST Open Repository, V1
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Description
Liquid-assisted atmospheric plasma polymerisation (LA-APP) enables the rapid curing of liquid monomer layers into polymer thin films without chemical initiators. This study investigates the plasma-induced free-radical polymerisation of trimethylolpropane propoxylate triacrylate (TMPTA-PO) to elucidate the role of liquid monomer layer thickness and plasma exposure on curing efficiency. Static and dynamic deposition approaches revealed a thickness-dependent diffusion depth of plasma-generated reactive species, with FTIR spectroscopy quantifying a high conversion degree for thin layers and incomplete bulk curing for thicker layers. The approach was implemented to embed rosmarinic acid as a natural antioxidant, yielding thin films with preserved antioxidant activity. These findings provide fundamental insight into plasma–liquid interactions and guidelines for controlled fabrication of multifunctional coatings. (2026-06-01)
***This entry has been automatically imported via OpenAlex by LIST harvest scripts. Please refer to https://doi.org/10.1002/ppap.70207 for the original and latest version of the publication*** (2026-07-01)
Subject Chemistry; Medicine, Health and Life Sciences; Physics
Keyword Monomer, Curing (chemistry), Polymerization, Plasma polymerization, Polymer, UV curing, Coating, Trimethylolpropane, Fourier transform infrared spectroscopy
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